Sector-Based Top-Down Estimates of NO _x , SO₂, and CO Emissions in East Asia.

ABSTRACT: Top-down estimates using satellite data provide important information on the sources of air pollutants. We develop a sector-based 4D-Var framework based on the GEOS-Chem adjoint model to address the impacts of co-emissions and chemical interactions on top-down emission estimates. We apply OMI NO₂, OMI SO₂, and MOPITT CO observations to estimate NO _x , SO₂, and CO emissions in East Asia during 2005-2012. Posterior evaluations with surface measurements show reduced normalized mean bias (NMB) by 7% (NO₂)-15% (SO₂) and normalized mean square error (NMSE) by 8% (SO₂)-9% (NO₂) compared to a species-based inversion. This new inversion captures the peak years of Chinese SO₂ (2007) and NO

SUBMITTER: Qu Z 

PROVIDER: S-EPMC9286828 | biostudies-literature | 2022 Jan

REPOSITORIES: biostudies-literature