Dataset Information

Heteroatom Modification Enhances Corrosion Durability in High-Mechanical-Performance Graphene-Reinforced Aluminum Matrix Composites.

ABSTRACT: The antagonism between strength and corrosion resistance in graphene-reinforced aluminum matrix composites is an inherent challenge to designing reliable structural components. Heteroatom microstructural modification is highly appreciated to conquer the obstacle. Here, a bottom-up strategy to exploit the heterogeneous phase interface to enable high corrosion durability is proposed. Deformation-driven metallurgy derived from severe plastic deformation is developed to produce Mg-alloyed fluorinated graphene structures with homogeneous dispersion. These structures allow for absorbing corrosion products, forming a dense protective layer against corrosion, and local micro-tuning of the suppression of charge transfer. This results in superior corrosion resistance with an outstanding strength-ductility balance of the composites via ultrafine-grained and precipitation strengthening. The anti-corrosion polarization resistance remains 89% of the initial state after 2-month immersion in chloride-containing environment, while the ultra-tensile strength and elongation of 532 ± 39 MPa and 17.3 ± 1.2% are obtained. The economical strategy of heteroatom modification broadens the horizon for anti-corrosion engineering in aluminum matrix composites, which is critical for the design of carbonaceous nanomaterial-reinforced composites to realize desired performances for practical applications.

SUBMITTER: Xie Y

PROVIDER: S-EPMC9376822 | biostudies-literature | 2022 Aug

REPOSITORIES: biostudies-literature

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Heteroatom Modification Enhances Corrosion Durability in High-Mechanical-Performance Graphene-Reinforced Aluminum Matrix Composites.

Xie Yuming Y Meng Xiangchen X Chang Yuexin Y Mao Dongxin D Qin Zhiwei Z Wan Long L Huang Yongxian Y

Advanced science (Weinheim, Baden-Wurttemberg, Germany) 20220615 23

The antagonism between strength and corrosion resistance in graphene-reinforced aluminum matrix composites is an inherent challenge to designing reliable structural components. Heteroatom microstructural modification is highly appreciated to conquer the obstacle. Here, a bottom-up strategy to exploit the heterogeneous phase interface to enable high corrosion durability is proposed. Deformation-driven metallurgy derived from severe plastic deformation is developed to produce Mg-alloyed fluorinate ...[more]

PMID: 35703130

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Project description:Metal matrix composites (MMCs) have wide applications due to being lightweight, their high strength, and immense resistance to wear. To explore new generation materials like aluminum-based metal matrix composites (AMCs) for wide engineering applications, the present work aimed at investigating the effect of changes in composition, sintering time, and temperature on the hardness and surface roughness of AMCs containing SiC and ZrSiO4 in wt % of 5, 20, 30, and 40 binary and hybrid sample pallets. The samples have been prepared by powder metallurgy (PM) method under 1000 psi pressure. After compaction, the above pallets sintered at different temperatures ranging from 500 °C to 1100 °C with an increment of 200 °C and 15 min intervals for four levels of temperature and time, respectively. Afterwards, sensitivity analysis has been done by investigating the effect of chemical composition, sintering time, and sintering temperature of the binary and hybrid composites on hardness and surface roughness. Morphological studies on the composites were carried out using field emission scanning electron microscope (FESEM) with energy dispersive spectroscopy (EDS). It has been observed that hardness is increased by increasing the sintering temperature in the case of SiC, whereas surface roughness did not change much by changing the composition. Additionally, a rise in temperature lead to liquid-state sintering. SEM images obtained during the elemental analysis showed that porosity is generated within the samples after sintering due to the higher melting point of reinforcements compared to a base metal, i.e., aluminum. Mathematical equations have also been developed via regression analysis using Minitab and excel for the confirmation and validation of experimental data. Analysis of Variance (ANOVA) has also been done, and its tables are shown and discussed in the paper. Hence, the most optimized findings relating the changes in the composition of reinforcements, sintering temperature, and sintering time (input variables) with porosity, hardness, and surface roughness have been presented in the current study.

Dataset Information

Heteroatom Modification Enhances Corrosion Durability in High-Mechanical-Performance Graphene-Reinforced Aluminum Matrix Composites.

Publications

Heteroatom Modification Enhances Corrosion Durability in High-Mechanical-Performance Graphene-Reinforced Aluminum Matrix Composites.

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