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Anomalous plasmons in a two-dimensional Dirac nodal-line Lieb lattice.

ABSTRACT: Plasmons in two-dimensional (2D) Dirac materials feature an interesting regime with a tunable frequency, and long propagating length and lifetime, but are rarely achieved in the visible light regime. Using a tight-binding (TB) model in combination with first-principles calculations, we investigated plasmon modes in a 2D Lieb lattice with a Dirac nodal-line electronic structure. In contrast to conventional 2D plasmons, anomalous plasmons in the Lieb lattice exhibit the unique features of a carrier-density-independent frequency, being Landau-damping free in a wide-range of wave vectors, a high frequency, and high subwavelength confinement. Remarkably, by using first-principles calculations, we proposed a candidate material, 2D Be₂C monolayer, to achieve these interesting plasmon properties. The plasmons in the Be₂C monolayer can survive up to the visible frequency region and propagate to large momentum transfer that has rarely been reported. The anomalous plasmons revealed in the Lieb lattice offer a promising platform for the study of 2D plasmons as well as the design of 2D plasmonic materials.

SUBMITTER: Ding C

PROVIDER: S-EPMC9419277 | biostudies-literature | 2021 Feb

REPOSITORIES: biostudies-literature

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Anomalous plasmons in a two-dimensional Dirac nodal-line Lieb lattice.

Ding Chao C Gao Han H Geng Wenhui W Zhao Mingwen M

Nanoscale advances 20201226 4

Plasmons in two-dimensional (2D) Dirac materials feature an interesting regime with a tunable frequency, and long propagating length and lifetime, but are rarely achieved in the visible light regime. Using a tight-binding (TB) model in combination with first-principles calculations, we investigated plasmon modes in a 2D Lieb lattice with a Dirac nodal-line electronic structure. In contrast to conventional 2D plasmons, anomalous plasmons in the Lieb lattice exhibit the unique features of a carrie ...[more]

PMID: 36133292

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Project description:Two-dimensional topological insulators (2D TIs) have distinct electronic properties that make them attractive for various applications, especially in spintronics. The conductive edge states in 2D TIs are protected from disorder and perturbations and are spin-polarized, which restrict current flow to a single spin orientation. In contrast, topological nodal line semimetals (TNLSM) are distinct from TIs because of the presence of a 1D ring of degeneracy formed from two bands that cross each other along a line in the Brillouin zone. These nodal lines are protected by topology and can be destroyed only by breaking certain symmetry conditions, making them highly resilient to disorder and defects. However, 2D TNLSMs do not possess protected boundary modes, which makes their investigation challenging. There have been several theoretical predictions of 2D TNLSMs, however, experimental realizations are rare. β-Sn, a metallic allotrope of tin with a superconducting temperature of 3.72 K, may be a candidate for a topological superconductor that can host Majorana Fermions for quantum computing. In this work, single layers of α-Sn and β-Sn on a Cu(111) substrate are successfully prepared and studied using scanning tunneling microscopy, angle-resolved photoemission spectroscopy, and density functional theory calculations. The lattice and electronic structure undergo a topological transition from 2D topological insulator α-Sn to 2D TNLSM β-Sn, with two types of nodal lines coexisting in monolayer β-Sn. Such a realization of two types of nodal lines in one 2D material has not been reported to date. Moreover, we also observed an unexpected phenomenon of freestanding-like electronic structures of β-Sn/Cu(111), highlighting the potential of ultrathin β-Sn films as a platform for exploring the electronic properties of 2D TNLSM and topological superconductors, such as few-layer superconducting β-Sn in lateral contact with topological nodal line single-layer β-Sn.

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Anomalous plasmons in a two-dimensional Dirac nodal-line Lieb lattice.

Publications

Anomalous plasmons in a two-dimensional Dirac nodal-line Lieb lattice.

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