Dataset Information

Integrated Assessment of Waste Tire Pyrolysis and Upgrading Pathways for Production of High-Value Products.

ABSTRACT: Waste tire pyrolysis has received increasing attention as a promising technology recently due to the shortage of fossil resources and the severity of environmental impact. In this study, the process of waste tire pyrolysis and upgrading to obtain high-value products was simulated by Aspen Plus. Also, based on life cycle assessment, the indexes of energy, environmental, economic, and comprehensive performance were proposed to evaluate different high-value pathways. Results demonstrate that the integrated system of waste tire pyrolysis, pyrolytic oil (TPO) refining, and pyrolytic carbon black (CBp) modification has higher energy efficiency than the independent system of TPO refining, with an improvement rate of 2.6%. Meanwhile, the resource-environmental performance of the integrated system is better. However, combined with the economic benefit, the independent system is more comprehensively beneficial, with the index of comprehensive performance (BEECR) of 0.94, which increases by 3.3% compared with the integrated system. Furthermore, the comparisons of different improved high-value paths based on the independent system as the benchmark indicate that the pathway of promoting sulfur conversion during pyrolysis to reduce the sulfur content in TPO can increase the BEECR from 0.94 to 1.064, with the growth of 13.2%. Also, the physical modification of CBp to reduce the production cost and environmental impact has better performance of BEECR, increasing by 20.2%. The final sensitivity analyses show that the combined improved high-value case established by the abovementioned two paths can achieve a favorable benefit in a wide range of crude oil and waste tire prices and the environmental tax.

SUBMITTER: Wu Q

PROVIDER: S-EPMC9453798 | biostudies-literature | 2022 Sep

REPOSITORIES: biostudies-literature

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Integrated Assessment of Waste Tire Pyrolysis and Upgrading Pathways for Production of High-Value Products.

Wu Qijing Q Zhang Qianqian Q Chen Xiaoyan X Song Guohui G Xiao Jun J

ACS omega 20220824 35

Waste tire pyrolysis has received increasing attention as a promising technology recently due to the shortage of fossil resources and the severity of environmental impact. In this study, the process of waste tire pyrolysis and upgrading to obtain high-value products was simulated by Aspen Plus. Also, based on life cycle assessment, the indexes of energy, environmental, economic, and comprehensive performance were proposed to evaluate different high-value pathways. Results demonstrate that the in ...[more]

PMID: 36092573

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Project description:Electronic waste (e-waste) generation has been growing in volume worldwide, and the diversity of its material composition is increasing. Sustainable management of this material is critical to achieving a circular-economy and minimizing environmental and public health risks. This study's objective was to investigate the use of pyrolysis as a possible technique to recover valuable materials and energy from different components of e-waste as an alternative approach for limiting their disposal to landfills. The study includes investigating the potential environmental impact of thermal processing of e-waste. The mass loss and change in e-waste chemicals during pyrolysis were also considered. The energy recovery from pyrolysis was made in a horizontal tube furnace under anoxic and isothermal conditions of selected temperatures of 300 °C, 400 °C, and 500 °C. Critical metals that include the rare earth elements and other metals (such as In, Co, Li) and valuable metals (Au, Ag, Pt group) were recovered from electronic components. Pyrolysis produced liquid and gas mixtures of organic compounds that can be used as fuels. Still, the process also emitted particulate matter and semi-volatile organic products, and the remaining ash contained leachable pollutants. Furthermore, toxicity characteristics leaching procedure (TCLP) of e-waste and partly oxidized products were conducted to measure the levels of pollutants leached before and after pyrolysis at selected temperatures. TCLP result revealed the presence of heavy metals like As, Cr, Cd, and Pd. Lead was found at 160 mg/L in PCBs leachate, which exceeded the toxicity characteristics (TC) limit of 5 mg/L. Liquid sample analysis from TCLP also showed the presence of C10-C19 components, including benzene. This study's results contribute to the development of practical recycling alternative approaches that could help reduce health risks and environmental problems and recover materials from e-waste. These results will also help assess the hazard risks that workers are exposed to semi-formal recycling centers.

Dataset Information

Integrated Assessment of Waste Tire Pyrolysis and Upgrading Pathways for Production of High-Value Products.

Publications

Integrated Assessment of Waste Tire Pyrolysis and Upgrading Pathways for Production of High-Value Products.

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