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Perturbation of clopyralid on bio-denitrification and nitrite accumulation: Long-term performance and biological mechanism.


ABSTRACT: The contaminant of herbicide clopyralid (3,6-dichloro-2- pyridine-carboxylic acid, CLP) poses a potential threat to the ecological system. However, there is a general lack of research devoted to the perturbation of CLP to the bio-denitrification process, and its biological response mechanism remains unclear. Herein, long-term exposure to CLP was systematically investigated to explore its influences on denitrification performance and dynamic microbial responses. Results showed that low-concentration of CLP (<15 mg/L) caused severe nitrite accumulation initially, while higher concentrations (35-60 mg/L) of CLP had no further effect after long-term acclimation. The mechanistic study demonstrated that CLP reduced nitrite reductase (NIR) activity and inhibited metabolic activity (carbon metabol

SUBMITTER: Sun S 

PROVIDER: S-EPMC9488107 | biostudies-literature | 2022 Jan

REPOSITORIES: biostudies-literature

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