A green and sustainable strategy toward lithium resources recycling from spent batteries.

ABSTRACT: Recycling lithium from spent batteries is challenging because of problems with poor purity and contamination. Here, we propose a green and sustainable lithium recovery strategy for spent batteries containing LiFePO₄, LiCoO₂, and LiNi_0.5Co_0.2Mn_0.3O₂ electrodes. Our proposed configuration of "lithium-rich electrode || LLZTO@LiTFSI+P3HT || LiOH" system achieves double-side and roll-to-roll recycling of lithium-containing electrode without destroying its integrity. The LiTFSI+P3HT-modified LLZTO membrane also solves the H⁺/Li⁺ exchange problem and realizes a waterproof protection of bare LLZTO in the aqueous working environment. On the basis of these advantages, our system shows high Li selectivity (97%) an

SUBMITTER: Xu J 

PROVIDER: S-EPMC9534500 | biostudies-literature | 2022 Oct

REPOSITORIES: biostudies-literature