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Solvent-Free Fabrication of Thick Electrodes in Thermoplastic Binders for High Energy Density Lithium-Ion Batteries.


ABSTRACT: The rapid development of electric vehicles has generated a recent demand for high energy density lithium-ion batteries (LIBs). One simple, effective way to enhance energy density of LIBs is to increase the thickness of electrodes. However, the conventional wet process used to fabricate thick electrodes involves the evaporation of large amounts of organic solvents, which causes an inhomogeneous distribution of conductive additives and binders. This weakens the mechanical and electrochemical network between active materials, resulting in poor electrochemical performance and structural degradation. Herein, we introduce a new strategy to produce homogeneous thick electrodes by using a dry, solvent-free process. Instead of using a conventional PVDF (polyvinylidene fluoride) binder, we employed

SUBMITTER: Kim HM 

PROVIDER: S-EPMC9565545 | biostudies-literature | 2022 Sep

REPOSITORIES: biostudies-literature