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Spray-coated perovskite hemispherical photodetector featuring narrow-band and wide-angle imaging.

ABSTRACT: Sphere imagers featuring specific wavelength recognition and wide-angle imaging are required to meet the fast development of modern technology. However, it is still challenging to deposit high-quality photosensitive layers on sphere substrates from low-cost solution processes. Here we report spray-coated quasi-two-dimensional phenylethylammonium/formamidinium lead halide (PEA₂FA_n-1Pb_nX_3n+1) perovskite hemispherical photodetectors. The crystallization speed is manipulated by perovskite compositions, and the film thickness can be controlled by spray-coating cycles and solution concentration from tens of nanometers to hundreds of micrometers with a fast velocity of 1.28 × 10^-4 cm³ s^-1. The lens-free hemispherical photodetectors allow light response at a wide incident angle of 180°. Simultaneously, the wavelength selective response from visible to the near-infrared range is achieved with full width at half maximums (FWHMs) of ~20 nm, comparable to single-crystal devices. Wide-angle and wavelength-selective imaging are also demonstrated, which can find potential applications in intelligent recognition and intraoperative navigated surgery.

SUBMITTER: Feng X

PROVIDER: S-EPMC9569351 | biostudies-literature | 2022 Oct

REPOSITORIES: biostudies-literature

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Spray-coated perovskite hemispherical photodetector featuring narrow-band and wide-angle imaging.

Feng Xiaopeng X He Yuhong Y Qu Wei W Song Jinmei J Pan Wanting W Tan Mingrui M Yang Bai B Wei Haotong H

Nature communications 20221015 1

Sphere imagers featuring specific wavelength recognition and wide-angle imaging are required to meet the fast development of modern technology. However, it is still challenging to deposit high-quality photosensitive layers on sphere substrates from low-cost solution processes. Here we report spray-coated quasi-two-dimensional phenylethylammonium/formamidinium lead halide (PEA2FAn-1PbnX3n+1) perovskite hemispherical photodetectors. The crystallization s ...[more]

PMID: 36243753

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Project description:Psoriasis is a common chronic inflammatory and hyperproliferative immune-mediated skin disorder. Narrow-band UVB (NB-UVB) phototherapy is a convenient first-line treatment of psoriasis, though the mechanisms underlying its efficacy have not been completely elucidated. In order to improve our understanding of NB-UVB phototherapy, gene expression profiling was used to characterize gene expression in lesional epidermis from psoriasis patients undergoing NB-UVB phototherapy. Increased expression of melanogenesis pathway genes was observed to be the earliest response. At the end of treatment, genes involved in diverse biological processes were affected, such as pigmentation, cell adhesion, ectodermal development and metabolism. The relationship between gene expression and treatment outcome was further studied using Partial Least Squares Discriminant Analysis (PLS-DA). Gene ontology analysis showed that genes responding to phototherapy and highly correlated to treatment outcome were involved in oxidation reduction, growth and mitochondria organization. In particular SPATA18, a key regulator of mitochondria quality, was found to be significantly downregulated in psoriasis, and its upregulation following phototherapy was required for optimal clinical improvement. Our data suggest that oxidation reduction is a critical event for the resolution of psoriatic plaques. Twelve patients diagnosed with plaque type psoriasis were recruited to the study. NB-UVB irradiation was administered to the whole body two to three times a week. Treatment comprising approximately 24 sessions was given during two to three months. A total of six 4 mm diameter punch biopsies were taken from lesions on each psoriasis patient: two prior to UV treatment (pre-UV), two at the middle stage of UV treatment (after about one month of treatment, mid-UV) and two before the last treatment session (post-UV). Twelve healthy age-, sex- and skin type-matched volunteers were also recruited and two punch biopsies were taken from the buttocks. RNA was extracted from Laser capture microdissected epidermis.

Dataset Information

Spray-coated perovskite hemispherical photodetector featuring narrow-band and wide-angle imaging.

Publications

Spray-coated perovskite hemispherical photodetector featuring narrow-band and wide-angle imaging.

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