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A Honeycomb-like Ammonium-Ion Fiber Battery with High and Stable Performance for Wearable Energy Storage.

ABSTRACT: Aqueous ammonium-ion batteries have attracted intense interest lately as promising energy storage systems due to the price advantage and fast charge/discharge capability of ammonium-ion redox reactions. However, the research on the strength and energy storage characteristics of ammonium-ion fiber batteries is still limited. In this study, an ammonium-ion fiber battery with excellent mechanical strength, flexibility, high specific capacity, and long cycle-life has been developed with a robust honeycomb-like ammonium vanadate@carbon nanotube (NH₄V₄O₁₀@CNT) cathode. The fiber electrode delivers a steady specific capacity of 241.06 mAh cm^-3 at a current of 0.2 mA. Moreover, a fiber full cell consisting of an NH₄V₄O₁₀@CNT cathode and a PANI@CNT anode exhibits a specific capacity of 7.27 mAh cm^-3 at a current of 0.3 mA and retains a high capacity retention of 72.1% after 1000 cycles. Meanwhile, it shows good flexibility and superior electrochemical performance after 500 times bending or at different deformation states. This work offers a reference for long-cycle, flexible fibrous ammonium-ion batteries.

SUBMITTER: Sun J

PROVIDER: S-EPMC9573061 | biostudies-literature | 2022 Oct

REPOSITORIES: biostudies-literature

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A Honeycomb-like Ammonium-Ion Fiber Battery with High and Stable Performance for Wearable Energy Storage.

Sun Jiangdong J Nie Wenqi W Xu Shuai S Gao Pengxiang P Sun Shuang S Zheng Xianhong X Hu Qiaole Q Xu Zhenzhen Z

Polymers 20221003 19

Aqueous ammonium-ion batteries have attracted intense interest lately as promising energy storage systems due to the price advantage and fast charge/discharge capability of ammonium-ion redox reactions. However, the research on the strength and energy storage characteristics of ammonium-ion fiber batteries is still limited. In this study, an ammonium-ion fiber battery with excellent mechanical strength, flexibility, high specific capacity, and long cycle-life has been developed with a robust hon ...[more]

PMID: 36236097

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Project description:Three installation-level lithium-ion battery (LIB) energy storage system (ESS) tests were conducted to the specifications of the UL 9540A standard test method [1]. Each test included a mocked-up initiating ESS unit rack and two target ESS unit racks installed within a standard size 6.06 m (20 ft) International Organization for Standardization (ISO) container. All tests were conducted with an identical LIB configuration. The initiating unit rack included nine modules (2,430 individual 18650 form factor cells) with a total capacity of 28.9 kWh. The target unit racks were loaded to one-third capacity of the initiating unit with nine partial modules and a total capacity of 9.6 kWh. All cells in the container were charged to 100% state-of-charge and none were electrically connected. Within the initiating mock-up unit, a flexible film heater was wrapped around an individual 18650 form factor cell. This instrumented 18650 cell was heated at a rate of 6°C/min to initiate thermal runaway. Test 1 was a baseline performance test and did not utilize any active fire suppression systems. Test 2 included a Novec 1230 system designed for an 8.3 vol% concentration discharged upon activation of two smoke detectors installed inside the container. Test 3 incorporated a dry pipe water suppression system to provide a uniform 20.8 mm/min (0.5 gpm/ft2) spray density delivered at the top of the ESS unit enclosures. Thermocouples were used to measure the cell temperatures in the initiating unit rack and module surface temperatures for the initiating unit and target unit racks. Thermocouples were located throughout the ISO container to measure gas temperatures and wall temperatures. Schmidt-Boelter heat flux gauges were installed to measure incident heat flux to each of the target unit racks as well as the walls adjacent to the initiating rack. Smoke detectors and smoke obscuration meters were used to identify the presence of smoke and characterize opacity of the smoke in the container. Various laboratory- and industrial-grade sensors were used to characterize the gas composition throughout container.

Dataset Information

A Honeycomb-like Ammonium-Ion Fiber Battery with High and Stable Performance for Wearable Energy Storage.

Publications

A Honeycomb-like Ammonium-Ion Fiber Battery with High and Stable Performance for Wearable Energy Storage.

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