Compositional Constraints are Vital for Atmospheric PM_2.5 Source Attribution over India.

ABSTRACT: India experiences some of the highest levels of ambient PM_2.5 aerosol pollution in the world. However, due to the historical dearth of in situ measurements, chemical transport models that are often used to estimate PM_2.5 exposure over the region are rarely evaluated. Here, we conduct a novel model comparison with speciated airborne measurements of fine aerosol, revealing large biases in the ammonium and nitrate simulations. To address this, we incorporate process-level changes to the model and use satellite observations from the Cross-track Infrared Sounder (CrIS) and the TROPOspheric Monitoring Instrument (TROPOMI) to constrain ammonia and nitrogen oxide emissions. The resulting simulation demonstrates significantly lower bias (NMB_Modified: 0.19; NMB_B

SUBMITTER: Pai SJ 

PROVIDER: S-EPMC9590233 | biostudies-literature | 2022 Oct

REPOSITORIES: biostudies-literature