Using coherent X-rays to follow dynamics in amorphous ices.

ABSTRACT: Amorphous solid water plays an important role in our overall understanding of water's phase diagram. X-ray scattering is an important tool for characterising the different states of water, and modern storage ring and XFEL facilities have opened up new pathways to simultaneously study structure and dynamics. Here, X-ray photon correlation spectroscopy (XPCS) was used to study the dynamics of high-density amorphous (HDA) ice upon heating. We follow the structural transition from HDA to low-density amorphous (LDA) ice, by using wide-angle X-ray scattering (WAXS), for different heating rates. We used a new type of sample preparation, which allowed us to study μm-sized ice layers rather than powdered bulk samples. The study focuses on the non-equilibrium dynamics during fast heating, spontaneou

SUBMITTER: Ladd-Parada M 

PROVIDER: S-EPMC9648632 | biostudies-literature | 2022 Nov

REPOSITORIES: biostudies-literature