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Performance and Enhancement of Various Fillers Guiding Vanadium (V) Bioremediation.

ABSTRACT: Bioremediation of vanadium (V) pollution in groundwater is an emerging topic. However, knowledge of V in a biogeochemical process is limited and long-term effective removal methods are lacking. V(V) remediation processes by various kinds of auxiliary fillers (maifanite-1, maifanite-2, volcanic rock, green zeolite and ceramsite), agricultural biomass and microbial enhancing were explored in this study. In tests without inocula, the V(V) removal efficiencies of ceramsite (inert filler) and maifanite-2 (active filler) were 84.9% and 60.5%, respectively. When inoculated with anaerobic sludge, 99.9% of V(V) could be removed with the synergistic performance of straw and maifanite-2. TOC (Total Organic Carbon), trace elements and three-dimensional fluorescence analyses confirmed that maifanite-2 was the most suitable among various fillers in biological V(V) removal systems with straw. This study provides a collaborative method (adsorption-biology) by using straw with maifanite-2 in V(V)-contaminated groundwater. The knowledge gained in this study will help develop permeable reactive barrier technology to repair polluted groundwater to put forward a reasonable, effective and sustainable environmental treatment strategy.

SUBMITTER: Hao L

PROVIDER: S-EPMC9691244 | biostudies-literature | 2022 Nov

REPOSITORIES: biostudies-literature

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Performance and Enhancement of Various Fillers Guiding Vanadium (V) Bioremediation.

Hao Liting L Li Lin L Wang Bangyan B Wang Xinli X Shi Jinkai J Shi Chen C Hao Xiaodi X

International journal of environmental research and public health 20221113 22

Bioremediation of vanadium (V) pollution in groundwater is an emerging topic. However, knowledge of V in a biogeochemical process is limited and long-term effective removal methods are lacking. V(V) remediation processes by various kinds of auxiliary fillers (maifanite-1, maifanite-2, volcanic rock, green zeolite and ceramsite), agricultural biomass and microbial enhancing were explored in this study. In tests without inocula, the V(V) removal efficiencies of ceramsite (inert filler) and maifani ...[more]

PMID: 36429645

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Project description:A series of composites based on epoxy resin filled with additives of natural origin were prepared to investigate the influence of such fillers on the properties of the epoxy compositions. For this purpose, the composites containing 5 and 10 wt.% of additive of natural origin were obtained using the dispersion of oak wood waste and peanut shells in bisphenol A epoxy resin cured with isophorone-diamine. The oak waste filler had been obtained during the assembly of the raw wooden floor. The performed studies include testing of samples prepared using unmodified and chemically modified additives. Chemical modification via mercerization and silanization was performed to increase the poor compatibility between the highly hydrophilic fillers of natural origin and the hydrophobic polymer matrix. Additionally, the introduction of NH2 groups to the structure of modified filler via 3-aminopropyltriethoxysilane, potentially takes a part in co-crosslinking with the epoxy resin. Fourier Transformed Infrared Spectroscopy (FT-IR), as well as Scanning Electron Microscopy (SEM), were carried out, to study the influence of performed chemical modification on the chemical structure and morphology of wood and peanut shell flour. SEM analyses showed significant changes in the morphology of compositions with chemically modified fillers, indicating improved adhesion of the resin to lignocellulosic waste particles. Moreover, a series of mechanical (hardness, tensile strength, flexural strength, compressive strength, and impact strength) tests were carried out, to assess the influence of the application of fillers of natural origin on the properties of epoxy compositions. All composites with lignocellulosic filler were characterized by higher compressive strength (64.2 MPa-5%U-OF, 66.4%-SilOF, 63.2-5%U-PSF, and 63.8-5%SilPSF, respectively), compared to the values recorded for the reference epoxy composition without lignocellulosic filler (59.0 MPa-REF). The highest compressive strength, among all tested samples, was recorded for the composite filled with 10 wt.% of unmodified oak flour (69.1 MPa-10%U-OF). Additionally, higher values of flexural and impact strength, concerning pure BPA-based epoxy resin, were recorded for the composites with oak filler (respectively, flexural strength: 73.8 MPa-5%U-OF and 71.5 MPa-REF; impact strength: 15.82 kJ/m2-5%U-OF, 9.15 kJ/m2-REF). Epoxy composites with such mechanical properties might be considered as broadly understood construction materials. Moreover, samples containing wood flour as a filler exhibit better mechanical properties compared to those with peanut shell flour (tensile strength for samples containing post-mercerization filler: 48.04 MPa and 40.54 MPa; while post-silanization 53.53 MPa and 42.74 MPa for compositions containing 5 wt.% of wood and peanut shell flour, respectively). At the same time, it was found that increasing the weight share of flour of natural origin in both cases resulted in the deterioration of mechanical properties.

Dataset Information

Performance and Enhancement of Various Fillers Guiding Vanadium (V) Bioremediation.

Publications

Performance and Enhancement of Various Fillers Guiding Vanadium (V) Bioremediation.

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