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High-throughput exploration of activity and stability for identifying photoelectrochemical water splitting materials.


ABSTRACT: The experimental high-throughput (HT) exploration for a suitable solar water splitting photoanode has greatly relied on photoactivity as the sole descriptor to identify a promising region within the searched composition space. Although activity is essential, it is not sufficient for describing the overall performance and excludes other pertinent criteria for photoelectrochemical (PEC) water splitting. Photostability in the form of (photo)electrocatalyst dissolution must be tracked to illustrate the intricate relation between activity and stability for multinary photoelectrocatalysts. To access these two important metrics simultaneously, an automated PEC scanning flow cell coupled to an inductively coupled plasma mass spectrometer (PEC-ICP-MS) was used to study an Fe-Ti-W-O thin film materi

SUBMITTER: Jenewein KJ 

PROVIDER: S-EPMC9710305 | biostudies-literature | 2022 Nov

REPOSITORIES: biostudies-literature