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Phyllanthus emblica Seed-Derived Hierarchically Porous Carbon Materials for High-Performance Supercapacitor Applications.

ABSTRACT: The electrical double-layer supercapacitance performance of the nanoporous carbons prepared from the Phyllanthus emblica (Amala) seed by chemical activation using the potassium hydroxide (KOH) activator is reported. KOH activation was carried out at different temperatures (700-1000 °C) under nitrogen gas atmosphere, and in a three-electrode cell set-up the electrochemical measurements were performed in an aqueous 1 M sulfuric acid (H2SO4) solution. Because of the hierarchical pore structures with well-defined micro- and mesopores, Phyllanthus emblica seed-derived carbon materials exhibit high specific surface areas in the range of 1360 to 1946 m2 g-1, and the total pore volumes range from 0.664 to 1.328 cm3 g-1. The sample with the best surface area performed admirably as the supercapacitor electrode-material, achieving a high specific capacitance of 272 F g-1 at 1 A g-1. Furthermore, it sustained 60% capacitance at a high current density of 50 A g-1, followed by a remarkably long cycle-life of 98% after 10,000 subsequent charging/discharging cycles, demonstrating the electrode's excellent rate-capability. These results show that the Phyllanthus emblica seed would have significant possibilities as a sustainable carbon-source for the preparing high-surface-area activated-carbons desired in high-energy-storage supercapacitors.

SUBMITTER: Shrestha LK

PROVIDER: S-EPMC9739855 | biostudies-literature | 2022 Nov

REPOSITORIES: biostudies-literature

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Phyllanthus emblica Seed-Derived Hierarchically Porous Carbon Materials for High-Performance Supercapacitor Applications.

Shrestha Lok Kumar LK Shahi Sabina S Gnawali Chhabi Lal CL Adhikari Mandira Pradhananga MP Rajbhandari Rinita R Pokharel Bhadra P BP Ma Renzhi R Shrestha Rekha Goswami RG Ariga Katsuhiko K

Materials (Basel, Switzerland) 20221123 23

The electrical double-layer supercapacitance performance of the nanoporous carbons prepared from the Phyllanthus emblica (Amala) seed by chemical activation using the potassium hydroxide (KOH) activator is reported. KOH activation was carried out at different temperatures (700-1000 °C) under nitrogen gas atmosphere, and in a three-electrode cell set-up the electrochemical measurements were performed in an aqueous 1 M sulfuric acid (H2SO4) solution. Because of the hie ...[more]

PMID: 36499823

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Project description:To address the growing energy demands of sustainable development, it is crucial to develop new materials that can improve the efficiency of energy storage systems. Hierarchically structured porous materials have shown their great potential for energy storage applications owing to their large accessible space, high surface area, low density, excellent accommodation capability with volume and thermal variation, variable chemical compositions and well controlled and interconnected hierarchical porosity at different length scales. Porous hierarchy benefits electron and ion transport, and mass diffusion and exchange. The electrochemical behavior of hierarchically structured porous materials varies with different pore parameters. Understanding their relationship can lead to the defined and accurate design of highly efficient hierarchically structured porous materials to enhance further their energy storage performance. In this review, we take the characteristic parameters of the hierarchical pores as the survey object to summarize the recent progress on hierarchically structured porous materials for energy storage. This is the first of this kind exclusively to survey the performance of hierarchically structured porous materials from different porous characteristics. For those who are not familiar with hierarchically structured porous materials, a series of very significant synthesis strategies of hierarchically structured porous materials are firstly and briefly reviewed. This will be beneficial for those who want to quickly obtain useful reference information about the synthesis strategies of new hierarchically structured porous materials to improve their performance in energy storage. The effect of different organizational, structural and geometric parameters of porous hierarchy on their electrochemical behavior is then deeply discussed. We outline the existing problems and development challenges of hierarchically structured porous materials that need to be addressed in renewable energy applications. We hope that this review can stimulate strong intuition into the design and application of new hierarchically structured porous materials in energy storage and other fields.

Dataset Information

Phyllanthus emblica Seed-Derived Hierarchically Porous Carbon Materials for High-Performance Supercapacitor Applications.

Publications

<i>Phyllanthus emblica</i> Seed-Derived Hierarchically Porous Carbon Materials for High-Performance Supercapacitor Applications.

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