High Multi-Environmental Mechanical Stability and Adhesive Transparent Ionic Conductive Hydrogels Used as Smart Wearable Devices.

ABSTRACT: Ionic conductive hydrogels used as flexible wearable sensor devices have attracted considerable attention because of their easy preparation, biocompatibility, and macro/micro mechanosensitive properties. However, developing an integrated conductive hydrogel that combines high mechanical stability, strong adhesion, and excellent mechanosensitive properties to meet practical requirements remains a great challenge owing to the incompatibility of properties. Herein, we prepare a multifunctional ionic conductive hydrogel by introducing high-modulus bacterial cellulose (BC) to form the skeleton of double networks, which exhibit great mechanical properties in both tensile (83.4 kPa, 1235.9% strain) and compressive (207.2 kPa, 79.9% strain) stress-strain tests. Besides, the fabricated hydrogels containing high-concentration Ca2+ show excellent anti-freezing (high ionic conductivities of 1.92 and 0.36 S/m at room temperature and -35 ∘C, respectively) properties. Furthermore, the sensing mechanism based on the conductive units and applied voltage are investigated to the benefit of the practical applications of prepared hydrogels. Therefore, the designed and fabricated hydrogels provide a novel strategy and can serve as candidates in the fields of sensors, ionic skins, and soft robots.

SUBMITTER: Wu Y 

PROVIDER: S-EPMC9739927 | biostudies-literature | 2022 Dec

REPOSITORIES: biostudies-literature