High-operating-temperature mid-infrared photodetectors via quantum dot gradient homojunction.

ABSTRACT: Due to thermal carriers generated by a narrow mid-infrared energy gap, cooling is always necessary to achieve ideal photodetection. In quantum dot (QD), the electron thermal generation should be reduced with quantum confinement in all three dimensions. As a result, there would be a great potential to realize high-operating-temperature (HOT) QD mid-IR photodetectors, though not yet achieved. Taking the advantages of colloidal nanocrystals' solution processability and precise doping control by surface dipoles, this work demonstrates a HOT mid-infrared photodetector with a QD gradient homojunction. The detector achieves background-limited performance with D^* = 2.7 × 10¹¹ Jones on 4.2 μm at 80 K, above 10¹¹ Jones until 200 K, above 10¹⁰ Jones until 2

SUBMITTER: Xue X 

PROVIDER: S-EPMC9805449 | biostudies-literature | 2023 Jan

REPOSITORIES: biostudies-literature