Understanding the Photoluminescence Quenching of Liquid Exfoliated WS₂ Monolayers.

ABSTRACT: Monolayer transition metal dichalcogenides (TMDs) are being investigated as active materials in optoelectronic devices due to their strong excitonic effects. While mechanical exfoliation (ME) of monolayer TMDs is limited to small areas, these materials can also be exfoliated from their parent layered materials via high-volume liquid phase exfoliation (LPE). However, it is currently considered that LPE-synthesized materials show poor optoelectronic performance compared to ME materials, such as poor photoluminescence quantum efficiencies (PLQEs). Here we evaluate the photophysical properties of monolayer-enriched LPE WS₂ dispersions via steady-state and time-resolved optical spectroscopy and benchmark these materials against untreated and chemically treated ME WS₂ monol

SUBMITTER: Li Z 

PROVIDER: S-EPMC9806825 | biostudies-literature | 2022 Dec

REPOSITORIES: biostudies-literature