Giant photon momentum locked THz emission in a centrosymmetric Dirac semimetal.

ABSTRACT: Strong second-order optical nonlinearities often require broken material centrosymmetry, thereby limiting the type and quality of materials used for nonlinear optical devices. Here, we report a giant and highly tunable terahertz (THz) emission from thin polycrystalline films of the centrosymmetric Dirac semimetal PtSe₂. Our PtSe₂ THz emission is turned on at oblique incidence and locked to the photon momentum of the incident pump beam. Notably, we find an emitted THz efficiency that is giant: It is two orders of magnitude larger than the standard THz-generating nonlinear crystal ZnTe and has values approaching that of the noncentrosymmetric topological material TaAs. Further, PtSe₂ THz emission displays THz sign and amplitude that is controlled by the incid

SUBMITTER: Cheng L 

PROVIDER: S-EPMC9812375 | biostudies-literature | 2023 Jan

REPOSITORIES: biostudies-literature