Magnetic correlations of iron oxide nanoparticles as probed by polarized SANS in stretched magnetic nanoparticle-elastomer composites.

ABSTRACT: We have investigated the magnetic correlations among 7 nm iron oxide nanoparticles embedded in stretched silicone elastomers using polarized Small Angle Neutron Scattering (SANS). The magnetic nanoparticle (MNP)-elastomer composite can be stretched during experiments, and macroscopic deformations cause rearrangement of the iron oxide particles on the nanoscale. Polarized neutrons can be used to nondestructively probe the arrangement of magnetic nanoparticles before and after stretching, so that the relationship between applied stress and nanoscale magnetization can be interrogated. We find that stretching the MNP-elastomer composite past a certain threshold dramatically changes the structural and magnetic morphology of the system. The unstretched sample is modeled well by ~40 nm clusters o

SUBMITTER: Oberdick SD 

PROVIDER: S-EPMC9813909 | biostudies-literature | 2022

REPOSITORIES: biostudies-literature