Effects of Rare Earth Metal Promotion over Zeolite-Supported Fe-Cu-Based Catalysts on the Light Olefin Production Performance in Fischer-Tropsch Synthesis.

ABSTRACT: Fischer-Tropsch synthesis (FTS), a significant reaction for effective H₂ utilization, is a promising approach for direct production of light olefins from syngas (H₂ + CO). For the FT-Olefin process, an efficient catalyst restricting the product distribution of FTS to light olefins is required. Aligned with this goal, we synthesized 24 catalysts comprising Fe and Cu in combination with rare earth metals (La, Ce, Nd, Ho, Er) and zeolite supports (ultrastable Y and mordenite). FT-Olefin performances of these catalysts were screened using a high-throughput test system at atmospheric pressure, and then promising catalysts were tested under high pressure in a conventional test system. Results show that Nd increases selectivity to light olefins and Ho suppresses C₅

SUBMITTER: Burgun U 

PROVIDER: S-EPMC9835664 | biostudies-literature | 2023 Jan

REPOSITORIES: biostudies-literature