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Distinct relaxation mechanism at room temperature in metallic glass.


ABSTRACT: How glasses relax at room temperature is still a great challenge for both experimental and simulation studies due to the extremely long relaxation time-scale. Here, by employing a modified molecular dynamics simulation technique, we extend the quantitative measurement of relaxation process of metallic glasses to room temperature. Both energy relaxation and dynamics, at low temperatures, follow a stretched exponential decay with a characteristic stretching exponent β = 3/7, which is distinct from that of supercooled liquid. Such aging dynamics originates from the release of energy, an intrinsic nature of out-of-equilibrium system, and manifests itself as the elimination of defects through localized atomic strains. This finding is also supported by long-time stress-relaxation experiments of various metallic glasses, confirming its validity and universality. Here, we show that the distinct relaxation mechanism can be regarded as a direct indicator of glass transition from a dynamic perspective.

SUBMITTER: Sun YT 

PROVIDER: S-EPMC9892575 | biostudies-literature | 2023 Feb

REPOSITORIES: biostudies-literature

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Distinct relaxation mechanism at room temperature in metallic glass.

Sun Yi-Tao YT   Zhao Rui R   Ding Da-Wei DW   Liu Yan-Hui YH   Bai Hai-Yang HY   Li Mao-Zhi MZ   Wang Wei-Hua WH  

Nature communications 20230201 1


How glasses relax at room temperature is still a great challenge for both experimental and simulation studies due to the extremely long relaxation time-scale. Here, by employing a modified molecular dynamics simulation technique, we extend the quantitative measurement of relaxation process of metallic glasses to room temperature. Both energy relaxation and dynamics, at low temperatures, follow a stretched exponential decay with a characteristic stretching exponent β = 3/7, which is distinct from  ...[more]

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