Coherent correlation imaging for resolving fluctuating states of matter.

ABSTRACT: Fluctuations and stochastic transitions are ubiquitous in nanometre-scale systems, especially in the presence of disorder. However, their direct observation has so far been impeded by a seemingly fundamental, signal-limited compromise between spatial and temporal resolution. Here we develop coherent correlation imaging (CCI) to overcome this dilemma. Our method begins by classifying recorded camera frames in Fourier space. Contrast and spatial resolution emerge by averaging selectively over same-state frames. Temporal resolution down to the acquisition time of a single frame arises independently from an exceptionally low misclassification rate, which we achieve by combining a correlation-based similarity metric^1,2 with a modified, iterative hierarchical clustering algorithm

SUBMITTER: Klose C 

PROVIDER: S-EPMC9908557 | biostudies-literature | 2023 Feb

REPOSITORIES: biostudies-literature