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Efficient and stable organic solar cells enabled by multicomponent photoactive layer based on one-pot polymerization.


ABSTRACT: Degradation of the kinetically trapped bulk heterojunction film morphology in organic solar cells (OSCs) remains a grand challenge for their practical application. Herein, we demonstrate highly thermally stable OSCs using multicomponent photoactive layer synthesized via a facile one-pot polymerization, which show the advantages of low synthetic cost and simplified device fabrication. The OSCs based on multicomponent photoactive layer deliver a high power conversion efficiency of 11.8% and exhibit excellent device stability for over 1000 h (>80% of their initial efficiency retention), realizing a balance between device efficiency and operational lifetime for OSCs. In-depth opto-electrical and morphological properties characterizations revealed that the dominant PM6-b-L15 block polymers with

SUBMITTER: Liu B 

PROVIDER: S-EPMC9944902 | biostudies-literature | 2023 Feb

REPOSITORIES: biostudies-literature