Overall Water Splitting by a SrTaO₂N-Based Photocatalyst Decorated with an Ir-Promoted Ru-Based Cocatalyst.

ABSTRACT: The development of narrow-bandgap photocatalysts for one-step-excitation overall water splitting (OWS) remains a critical challenge in the field of solar hydrogen production. SrTaO₂N is a photocatalytic material having a band structure suitable for OWS under visible light (λ ≤ 600 nm). However, the presence of defects in the oxynitride and the lack of cocatalysts to promote simultaneous hydrogen and oxygen evolution make it challenging to realize OWS using this material. The present work demonstrates a SrTaO₂N-based particulate photocatalyst for OWS. This photocatalyst, which was composed of single crystals, was obtained by nitriding SrCl₂ and Ta₂O₅ together with NaOH, with the latter added to control the formation of defects. The subs

SUBMITTER: Chen K 

PROVIDER: S-EPMC9952422 | biostudies-literature | 2023 Jan

REPOSITORIES: biostudies-literature