Tunable interlayer excitons and switchable interlayer trions via dynamic near-field cavity.

ABSTRACT: Emerging photo-induced excitonic processes in transition metal dichalcogenide (TMD) heterobilayers, e.g., interplay of intra- and inter-layer excitons and conversion of excitons to trions, allow new opportunities for ultrathin hybrid photonic devices. However, with the associated large degree of spatial heterogeneity, understanding and controlling their complex competing interactions in TMD heterobilayers at the nanoscale remains a challenge. Here, we present an all-round dynamic control of interlayer-excitons and -trions in a WSe₂/Mo_0.5 W_0.5 Se₂ heterobilayer using multifunctional tip-enhanced photoluminescence (TEPL) spectroscopy with <20 nm spatial resolution. Specifically, we demonstrate the bandgap tunable interlayer excitons and the dynamic

SUBMITTER: Koo Y 

PROVIDER: S-EPMC9981773 | biostudies-literature | 2023 Mar

REPOSITORIES: biostudies-literature