Enhancement of Amplified Spontaneous Emission by Electric Field in CsPbBr₃ Perovskites.

ABSTRACT: Perovskite gain materials can sustain continuous-wave lasing at room-temperature. A first step toward the unachieved goal of electrically excited lasing would be an improvement in gain when electrical stimulation is added to the optical. However, to date, electrical stimulation supplementing optical has reduced gain performance. We find that amplified spontaneous emission (ASE) in a CsPbBr₃ perovskite light-emitting diode (LED) held under invariant subthreshold optical excitation can be turned on/off by the addition/removal of an electric field. A positive bias voltage leads to a factor of 3 reduction in the optical ASE threshold, the cause of which can be attributed to an enhancement of the radiative rate. The slow components (10 s time scale) of the modulation in the photolumi

SUBMITTER: Li Y 

PROVIDER: S-EPMC9999453 | biostudies-literature | 2023 Mar

REPOSITORIES: biostudies-literature