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Microcavity controlled coupling of excitonic qubits.

ABSTRACT: Controlled non-local energy and coherence transfer enables light harvesting in photosynthesis and non-local logical operations in quantum computing. This process is intuitively pictured by a pair of mechanical oscillators, coupled by a spring, allowing for a reversible exchange of excitation. On a microscopic level, the most relevant mechanism of coherent coupling of distant quantum bits--like trapped ions, superconducting qubits or excitons confined in semiconductor quantum dots--is coupling via the electromagnetic field. Here we demonstrate the controlled coherent coupling of spatially separated quantum dots via the photon mode of a solid state microresonator using the strong exciton-photon coupling regime. This is enabled by two-dimensional spectroscopy of the sample's coherent response, a sensitive probe of the coherent coupling. The results are quantitatively understood in a rigorous description of the cavity-mediated coupling of the quantum dot excitons. This mechanism can be used, for instance in photonic crystal cavity networks, to enable a long-range, non-local coherent coupling.

PROVIDER: S-EPMC3644086 | BioStudies | 2013-01-01T00:00:00Z

REPOSITORIES: biostudies

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Dynamically controlling the emission of single excitons in photonic crystal cavities.

Project description:Single excitons in semiconductor microcavities represent a solid state and scalable platform for cavity quantum electrodynamics, potentially enabling an interface between flying (photon) and static (exciton) quantum bits in future quantum networks. While both single-photon emission and the strong coupling regime have been demonstrated, further progress has been hampered by the inability to control the coherent evolution of the cavity quantum electrodynamics system in real time, as needed to produce and harness charge-photon entanglement. Here using the ultrafast electrical tuning of the exciton energy in a photonic crystal diode, we demonstrate the dynamic control of the coupling of a single exciton to a photonic crystal cavity mode on a sub-nanosecond timescale, faster than the natural lifetime of the exciton. This opens the way to the control of single-photon waveforms, as needed for quantum interfaces, and to the real-time control of solid-state cavity quantum electrodynamics systems.

2014-01-01 | S-EPMC4275591 | BioStudies

An exciton-polariton laser based on biologically produced fluorescent protein.

Project description:Under adequate conditions, cavity polaritons form a macroscopic coherent quantum state, known as polariton condensate. Compared to Wannier-Mott excitons in inorganic semiconductors, the localized Frenkel excitons in organic emitter materials show weaker interaction with each other but stronger coupling to light, which recently enabled the first realization of a polariton condensate at room temperature. However, this required ultrafast optical pumping, which limits the applications of organic polariton condensates. We demonstrate room temperature polariton condensates of cavity polaritons in simple laminated microcavities filled with biologically produced enhanced green fluorescent protein (eGFP). The unique molecular structure of eGFP prevents exciton annihilation even at high excitation densities, thus facilitating polariton condensation under conventional nanosecond pumping. Condensation is clearly evidenced by a distinct threshold, an interaction-induced blueshift of the condensate, long-range coherence, and the presence of a second threshold at higher excitation density that is associated with the onset of photon lasing.

1000-01-01 | S-EPMC4991930 | BioStudies

On-chip deterministic operation of quantum dots in dual-mode waveguides for a plug-and-play single-photon source.

Project description:A deterministic source of coherent single photons is an enabling device for quantum information processing. Quantum dots in nanophotonic structures have been employed as excellent sources of single photons with the promise of scaling up towards multiple photons and emitters. It remains a challenge to implement deterministic resonant optical excitation of the quantum dot required for generating coherent single photons, since residual light from the excitation laser should be suppressed without compromising source efficiency and scalability. Here, we present a planar nanophotonic circuit that enables deterministic pulsed resonant excitation of quantum dots using two orthogonal waveguide modes for separating the laser and the emitted photons. We report a coherent and stable single-photon source that simultaneously achieves high-purity (g<sup>(2)</sup>(0)?=?0.020?±?0.005), high-indistinguishability (V?=?96?±?2%), and >80% coupling efficiency into the waveguide. Such 'plug-and-play' single-photon source can be integrated with on-chip optical networks implementing photonic quantum processors.

2020-01-01 | S-EPMC7391626 | BioStudies

Quantum dot-embedded microspheres for remote refractive index sensing.

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Cavity Control of Excitons in Two-Dimensional Materials.

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2019-01-01 | S-EPMC6674266 | BioStudies

Strongly coupled slow-light polaritons in one-dimensional disordered localized states.

Project description:Cavity quantum electrodynamics advances the coherent control of a single quantum emitter with a quantized radiation field mode, typically piecewise engineered for the highest finesse and confinement in the cavity field. This enables the possibility of strong coupling for chip-scale quantum processing, but till now is limited to few research groups that can achieve the precision and deterministic requirements for these polariton states. Here we observe for the first time coherent polariton states of strong coupled single quantum dot excitons in inherently disordered one-dimensional localized modes in slow-light photonic crystals. Large vacuum Rabi splittings up to 311 ?eV are observed, one of the largest avoided crossings in the solid-state. Our tight-binding models with quantum impurities detail these strong localized polaritons, spanning different disorder strengths, complementary to model-extracted pure dephasing and incoherent pumping rates. Such disorder-induced slow-light polaritons provide a platform towards coherent control, collective interactions, and quantum information processing.

2013-01-01 | S-EPMC3683671 | BioStudies

Nanophotonic coherent light-matter interfaces based on rare-earth-doped crystals.

Project description:Quantum light-matter interfaces connecting stationary qubits to photons will enable optical networks for quantum communications, precise global time keeping, photon switching and studies of fundamental physics. Rare-earth-ion-doped crystals are state-of-the-art materials for optical quantum memories and quantum transducers between optical photons, microwave photons and spin waves. Here we demonstrate coupling of an ensemble of neodymium rare-earth-ions to photonic nanocavities fabricated in the yttrium orthosilicate host crystal. Cavity quantum electrodynamics effects including Purcell enhancement (F=42) and dipole-induced transparency are observed on the highly coherent (4)I(9/2)-(4)F(3/2) optical transition. Fluctuations in the cavity transmission due to statistical fine structure of the atomic density are measured, indicating operation at the quantum level. Coherent optical control of cavity-coupled rare-earth ions is performed via photon echoes. Long optical coherence times (T2?100??s) and small inhomogeneous broadening are measured for the cavity-coupled rare-earth ions, thus demonstrating their potential for on-chip scalable quantum light-matter interfaces.

1000-01-01 | S-EPMC4647856 | BioStudies

Quantum-state transfer from an ion to a photon.

Project description:One model for quantum networks1,2 is based on the probabilistic measurement of two photons, each entangled with a distant node, e.g., an atom or atomic ensemble3-7. A second, deterministic model transfers information directly from an atom onto a cavity photon, which carries it to a second node8, as recently demonstrated with neutral atoms9. In both cases, the challenge is to transfer information efficiently while preserving coherence. Here, following the second scheme, we map the quantum state of an ion onto a photon within an optical cavity. Using an ion enables deterministic state initialization10,11, while the cavity provides coherent coupling to a well-defined output mode12-15. Although it is often assumed that a cavity-based quantum interface requires the strong-coupling regime, we show transfer fidelities of 92% in the presence of non-negligible decoherence and characterize the interplay between fidelity and efficiency. Our time-independent mapping process offers a promising route toward ion-based quantum networks.

| S-EPMC3694356 | BioStudies

Coherent microwave-photon-mediated coupling between a semiconductor and a superconducting qubit.

Project description:Semiconductor qubits rely on the control of charge and spin degrees of freedom of electrons or holes confined in quantum dots. They constitute a promising approach to quantum information processing, complementary to superconducting qubits. Here, we demonstrate coherent coupling between a superconducting transmon qubit and a semiconductor double quantum dot (DQD) charge qubit mediated by virtual microwave photon excitations in a tunable high-impedance SQUID array resonator acting as a quantum bus. The transmon-charge qubit coherent coupling rate (~21?MHz) exceeds the linewidth of both the transmon (~0.8?MHz) and the DQD charge qubit (~2.7?MHz). By tuning the qubits into resonance for a controlled amount of time, we observe coherent oscillations between the constituents of this hybrid quantum system. These results enable a new class of experiments exploring the use of two-qubit interactions mediated by microwave photons to create entangled states between semiconductor and superconducting qubits.

2019-01-01 | S-EPMC6614454 | BioStudies

Manipulating nonlinear emission and cooperative effect of CdSe/ZnS quantum dots by coupling to a silver nanorod complex cavity.

Project description:Colloidal semiconductor quantum dots have three-dimensional confined excitons with large optical oscillator strength and gain. The surface plasmons of metallic nanostructures offer an efficient tool to enhance exciton-exciton coupling and excitation energy transfer at appropriate geometric arrangement. Here, we report plasmon-mediated cooperative emissions of approximately one monolayer of ensemble CdSe/ZnS quantum dots coupled with silver nanorod complex cavities at room temperature. Power-dependent spectral shifting, narrowing, modulation, and amplification are demonstrated by adjusting longitudinal surface plasmon resonance of silver nanorods, reflectivity and phase shift of silver nanostructured film, and mode spacing of the complex cavity. The underlying physical mechanism of the nonlinear excitation energy transfer and nonlinear emissions are further investigated and discussed by using time-resolved photoluminescence and finite-difference time-domain numerical simulations. Our results suggest effective strategies to design active plasmonic complex cavities for cooperative emission nanodevices based on semiconductor quantum dots.

1000-01-01 | S-EPMC4007083 | BioStudies

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