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3D Printed Nitrogen-Doped Thick Carbon Architectures for Supercapacitor: Ink Rheology and Electrochemical Performance.


ABSTRACT: The 3D printing technique offers huge opportunities for customized thick-electrode designs with high loading densities to enhance the area capacity in a limited space. However, key challenges remain in formulating 3D printable inks with exceptional rheological performance and facilitating electronic/ion transport in thick bulk electrodes. Herein, a hybrid ink consisting of woody-derived cellulose nanofibers (CNFs), multiwalled carbon nanotubes (MWCNTs), and urea is formulated for the 3D printing nitrogen-doped thick electrodes, in which CNFs serve as both dispersing and thickening agents for MWCNTs, whereas urea acts as a doping agent. By systematically tailoring the concentration-dependent rheological performance and 3D printing process of the ink, a variety of gel architectures with high

SUBMITTER: Zhou G 

PROVIDER: S-EPMC10074055 | biostudies-literature | 2023 Apr

REPOSITORIES: biostudies-literature