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Tuning the Defects of Two-Dimensional Layered Carbon/TiO2 Superlattice Composite for a Fast Lithium-Ion Storage.


ABSTRACT: Defect engineering is one of the effective ways to improve the electrochemical property of electrode materials for lithium-ion batteries (LIB). Herein, an organic functional molecule of p-phenylenediamine is embedded into two-dimensional (2D) layered TiO2 as the electrode for LIB. Then, the 2D carbon/TiO2 composites with the tuning defects are prepared by precise control of the polymerization and carbothermal atmospheres. Low valence titanium in metal oxide and nitrogen-doped carbon nanosheets can be obtained in the carbon/TiO2 composite under a carbonization treatment atmosphere of N2/H2 gas, which can not only increase the electronic conductivity of the material but also provide sufficient electrochemical active sites, thus producing an excellent rate capability and long-term cycle stabi

SUBMITTER: Liu B 

PROVIDER: S-EPMC8911284 | biostudies-literature | 2022 Feb

REPOSITORIES: biostudies-literature