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Surface plasmons induce topological transition in graphene/α-MoO3 heterostructures.


ABSTRACT: Polaritons in hyperbolic van der Waals materials-where principal axes have permittivities of opposite signs-are light-matter modes with unique properties and promising applications. Isofrequency contours of hyperbolic polaritons may undergo topological transitions from open hyperbolas to closed ellipse-like curves, prompting an abrupt change in physical properties. Electronically-tunable topological transitions are especially desirable for future integrated technologies but have yet to be demonstrated. In this work, we present a doping-induced topological transition effected by plasmon-phonon hybridization in graphene/α-MoO3 heterostructures. Scanning near-field optical microscopy was used to image hybrid polaritons in graphene/α-MoO3. We demonstrate the topological transition and characterize hybrid modes, which can be tuned from surface waves to bulk waveguide modes, traversing an exceptional point arising from the anisotropic plasmon-phonon coupling. Graphene/α-MoO3 heterostructures offer the possibility to explore dynamical topological transitions and directional coupling that could inspire new nanophotonic and quantum devices.

SUBMITTER: Ruta FL 

PROVIDER: S-EPMC9240047 | biostudies-literature | 2022 Jun

REPOSITORIES: biostudies-literature

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Surface plasmons induce topological transition in graphene/α-MoO<sub>3</sub> heterostructures.

Ruta Francesco L FL   Kim Brian S Y BSY   Sun Zhiyuan Z   Rizzo Daniel J DJ   McLeod Alexander S AS   Rajendran Anjaly A   Liu Song S   Millis Andrew J AJ   Hone James C JC   Basov D N DN  

Nature communications 20220628 1


Polaritons in hyperbolic van der Waals materials-where principal axes have permittivities of opposite signs-are light-matter modes with unique properties and promising applications. Isofrequency contours of hyperbolic polaritons may undergo topological transitions from open hyperbolas to closed ellipse-like curves, prompting an abrupt change in physical properties. Electronically-tunable topological transitions are especially desirable for future integrated technologies but have yet to be demons  ...[more]

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