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One-dimensional polaritons with size-tunable and enhanced coupling strengths in semiconductor nanowires.


ABSTRACT: Strong coupling of light with excitons in direct bandgap semiconductors leads to the formation of composite photonic-electronic quasi-particles (polaritons), in which energy oscillates coherently between the photonic and excitonic states with the vacuum Rabi frequency. The light-matter coherence is maintained until the oscillator dephases or the photon escapes. Exciton-polariton formation has enabled the observation of Bose-Einstein condensation in the solid-state, low-threshold polariton lasing and is also useful for terahertz and slow-light applications. However, maintaining coherence for higher carrier concentration and temperature applications still requires increased coupling strengths. Here, we report on size-tunable, exceptionally high exciton-polariton coupling strengths characterized by a vacuum Rabi splitting of up to 200 meV as well as a reduction in group velocity, in surface-passivated, self-assembled semiconductor nanowire cavities. These experiments represent systematic investigations on light-matter coupling in one-dimensional optical nanocavities, demonstrating the ability to engineer light-matter coupling strengths at the nanoscale, even in non-quantum-confined systems, to values much higher than in bulk.

SUBMITTER: van Vugt LK 

PROVIDER: S-EPMC3121826 | biostudies-literature | 2011 Jun

REPOSITORIES: biostudies-literature

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One-dimensional polaritons with size-tunable and enhanced coupling strengths in semiconductor nanowires.

van Vugt Lambert K LK   Piccione Brian B   Cho Chang-Hee CH   Cho Chang-Hee CH   Nukala Pavan P   Agarwal Ritesh R  

Proceedings of the National Academy of Sciences of the United States of America 20110531 25


Strong coupling of light with excitons in direct bandgap semiconductors leads to the formation of composite photonic-electronic quasi-particles (polaritons), in which energy oscillates coherently between the photonic and excitonic states with the vacuum Rabi frequency. The light-matter coherence is maintained until the oscillator dephases or the photon escapes. Exciton-polariton formation has enabled the observation of Bose-Einstein condensation in the solid-state, low-threshold polariton lasing  ...[more]

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