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Asymmetric Synthesis of Axinellamines A and B.

ABSTRACT: Axinellamines A and B are broad-spectrum antibacterial pyrrole-imidazole alkaloids that have a complex polycyclic skeleton. A new asymmetric synthesis of these marine sponge metabolites is described herein, featuring an oxidative rearrangement and an anchimeric chlorination reaction.

SUBMITTER: Ma Z 

PROVIDER: S-EPMC4836294 | biostudies-literature | 2016 Apr

REPOSITORIES: biostudies-literature

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Asymmetric Synthesis of Axinellamines A and B.

Ma Zhiqiang Z   Wang Xiao X   Ma Yuyong Y   Chen Chuo C  

Angewandte Chemie (International ed. in English) 20160308 15

Axinellamines A and B are broad-spectrum antibacterial pyrrole-imidazole alkaloids that have a complex polycyclic skeleton. A new asymmetric synthesis of these marine sponge metabolites is described herein, featuring an oxidative rearrangement and an anchimeric chlorination reaction. ...[more]

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